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All-Optical and Ultrafast Control of High-Order Exciton-Polariton Orbital Modes.

Created on 12 May 2025

Authors

Yuyang Zhang, Xin Zeng, Wenna Du, Zhiyong Zhang, Yuexing Xia, Jiepeng Song, Jianhui Fu, Shuai Zhang, Yangguang Zhong, Yubo Tian, Yiyang Gong, Shuai Yue, Yuanyuan Zheng, Xiaotian Bao, Yutong Zhang, Qing Zhang, Xinfeng Liu

Published in

Nano letters. May 11, 2025. Epub May 11, 2025.

Abstract

Exciton-polaritons flows within closed quantum circuits can spontaneously form phase-locked modes that carry orbital angular momentum (OAM). With its infinite set of angular momentum quantum numbers (), high-order OAM represents a transformative solution to the bandwidth bottleneck in multiplexed optical communication. However, its practical application is hindered by the limited choice of materials which in general requires cryogenic temperatures and the reliance on mechanical switching. In this work, we achieve stable and high-order (up to order of 33) OAM modes by constructing a closed quantum circuit using the halide perovskite microcavities at room temperature. By controlling the spatial and temporal symmetry of the closed quantum circuits using another laser pulse, we achieve significant tuning OAM of EP flows from 8 to 12. Our work demonstrates all-optical and ultrafast control of high-order OAM using exciton-polariton condensates in perovskite microcavities that would have important applications in high-throughput optical communications.

PMID:
40349216
Bibliographic data and abstract were imported from PubMed on 12 May 2025.

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