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Polarization-State-Dependent Charge Screening in Metal-Ferroelectric-Metal Memcapacitors Enabled by an IGZO Oxygen Reservoir Layer.

Created on 01 Jul 2026

Authors

Donghyeon Kim, Huiseong Shin, Junseok Kim, Hyeonjung Park, Changwoo Han, Myeongjae Choi, Changhwan Shin

Published in

ACS applied materials & interfaces. Jul 01, 2026. Epub Jul 01, 2026.

Abstract

An indium-gallium-zinc oxide (IGZO) oxygen reservoir layer (ORL) was introduced at the bottom interface of W/Hf0.5Zr0.5O2 (HZO)/W memcapacitors to induce asymmetric capacitance modulation without relying on domain pinning. The IGZO layer exhibits a polarization-state-dependent capacitance response, transitioning between a limited-screening state and an efficient-screening state during the bias sweep, which modulates the charge-screening response of the stack. This polarization-state-dependent charge-screening response results in asymmetric capacitance peaks during polarization switching and enables a significantly enhanced capacitance memory window (CMW). Equivalent circuit analysis quantitatively reveals the contribution of the IGZO layer and confirms its role in governing the observed C-V asymmetry. Systematic variation of stack configuration and IGZO thickness demonstrates that a bottom-interfaced, thickness-optimized IGZO layer maximizes both asymmetry and CMW. In addition, the IGZO layer functions as an oxygen reservoir, suppressing oxygen-vacancy-induced degradation and improving endurance. The device further exhibits stable analog synaptic characteristics, and a retention-aware state pruning strategy is introduced to mitigate retention-induced degradation, preserving read margin and improving computational accuracy under noise-aware conditions. These results establish IGZO-integrated MFM memcapacitors as a viable platform for high-performance ferroelectric capacitive memory and neuromorphic systems.

PMID:
42384435
Bibliographic data and abstract were imported from PubMed on 01 Jul 2026.

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